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In the entangled regime, one can consider the diffusion of primitive path points that, on time scales smaller than the reptation time, probes higher modes, which, according to the reptation model, should correspond to the relaxation times ~ ~ with integer j [we have first encountered this spectrum for the reptation model in (4153) where, due to uniform initial conditions, only odd values of j contribute] A further check of the crossover picture from unentangled to entangled behavior can be obtained from the molecular-weight dependence of the center-of-mass diffusion coefficient The time dependent segment diffusion allows us to test reptation ideas, including short-time features that are considered to be typical for reptation but are not described by the equations for the reptation model given in Section 432.

f (kHz)

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Modal Filtering. Various devices decrease the number of propagating modes in an optical system. A pinhole is the most common example. We have used pinholes several times to select a single spherical wave from a broader eld distribution, most recently in our discussion of the two-pinhole interferometer. Such devices are called spatial lters. As discussed in 9, spatial lters are commonly used in spectroscopy to break degeneracies between spectral and spatial degrees of freedom. Complex spatial lters may be implemented using diffractive devices or coded apertures. In the example of Fig. 6.25, spatial ltering may consist simply of discarding the light on one of the output arms. In that case, we have combined two input modes into one output mode. Absorption. A device that differentially absorbs some of the light in an optical system breaks time reversal symmetry and restructures the coherent modes. Modal Decorrelation. Modes propagate on different paths through the optical system. If the structure of the optical system is time varying on these paths, the relative coherence of the modes may be destroyed. The most common example is propagation through turbulence. In the example of Fig. 6.25, the two output beams may experience different time-varying phase modulation. Such modulation can render the output beams relatively incoherent, which diagonalizes J. In the case of the 50/50 beamsplitter with incoherent input beams, this produces relatively incoherent output beams with equal irradiances of (I1 I2 )=2.

In this section, we have learned how the analysis of equilibrium molecular dynamics simulationsis guided by the ideas of beyond-equilibrium statistical mechanics and thermodynamics The simulation results need to be analyzed in the light of a coarsegrained model Also for traditional equilibrium simulations, the search for reptation has led researchers to study coarse-grained polymer conformations and to look for diffusion within tubes86 However, the thermodynamically guided simulations go much further by using nonequilibrium ensembles defined in terms of coarse-grained variables, as explained for the rarefied Lennard-Jones gas in Section 845 Far beyond equilibrium, the use,of a fixed parameter <,such as the ratio of spring constants used to adjust the number of entanglements at equilibrium, is no longer satisfactory.

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