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and evaluation examining the majority of simple oxides demonstrated that a wide range of basic oxides can be effective The most active catalysts are the nonreducible Group IIA metal oxides 11,312 Other good catalysts are supported alkali oxides 313 ,314 and carbonates 91,315 It was also observed that Group IIA oxides, when promoted with Group IA cations, gave increased activity and selectivity 16,317 Chloride salts and chlorine compounds have similar beneficial effects 18-322 Certain lanthanide sesquioxides (La203, Sm203) also show considerable activity in converting methane to C2 hydrocarbons 23-327 These catalysts function optimally in the temperature range 650-800 C The products observed in the reaction are C2H6, C 2H4, CO, CO 2, H2, H20, and some higher hydrocarbons CH30H and CH 20 are also found in trace amounts Many of these oxides give remarkably similar conversion-selectivity results, suggesting a common active site and reaction mechanism.

( 11.36)

It was also found that the C2 selectivity decreases almost linearly with increasing methane conversion, usually achieved by increasing the oxygen concentration in the feed This is formulated as the "100% rule,,,295 indicating that methane conversion and C 2 selectivity roughly sum to 100% At low conversions, using reaction mixtures of high C~ : O2 ratio, selectivities of ::;70% may be obtained In fixed-bed flow reactors a C2 selectivity of 50% may be achieved at a conversion level of 40% at atmospheric pressure 12 C2 yields in the range 20-25% are usually achieved A C2 yield slightly better than 50% (80% selectivity at 65% methane conversion, above 700 C, Sm203 catalyst), however, has been reported 28 A special technique, a separative chemical reactor simulating a countercurrent chromatographic moving bed has been applied.

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Another technical modification has resulted in even higher yields 29 In this case methane coupling is carried out in a gas recycle electrocatalytic or catalytic reactor over silver catalysts (800 C, Ag on Y20rZr02 or Ag on Sm203 doped with CaO) and the recycle gas passes through a Linde 5A molecular sieve at 30 C The adsorbed C2 hydrocarbons, which are trapped and therefore protected from further oxidation, are subsequently desorbed at 400 C The method ensures high yields and selectivities (total yields up to 88%, ethylene yields ::;85%, ethylene selectivities ::;88% for methane conversion ::;97%) At present, there is a general agreement that the primary function of the catalysts in oxidative coupling of methane is to form methyl radicals.

import import import import flash.display.BitmapData; flash.geom.Matrix; flash.geom.Point; flash.geom.Rectangle;

Considerable evidence attained by electron paramagnetic resonance,313,330 mass spectroscopy,331 and isotopic labeling studies332-334 indicates that methyl radicals produced in a heterogeneous process are the primary intermediate in the production of ethane Methyl radicals are formed in a direct route with the involvement of surface oxygen (Os -) [Eq (328)] Alternatively, an acid-base process with the interaction of oxygen ions of low coordination number (0;-) with methane may form a methyl anion that then reacts further with molecular oxygen to give methyl radica1335-337 [Eq (329)]:.

1. In Layout mode, choose the layout to which you want to add the element. 2. Use the Fill, Border, Effects, and Line Width palettes to select the appropriate formatting for the new element. As an alternative, you can set the object s properties after you create it, if you want.

If[Get(ScriptParameter) = Utility::gSortField] Set Field[Utility::gSortOrder; Abs(Utility::gSortOrder 1)] Else Set Field[Utility::gSortField; Get(ScriptParameter)] Set Field[Utility::gSortOrder; Abs(Get(ActiveModifierKeys)-2) = 1] End If Sort Records [Restore; No dialog]

use Text::CSV_XS; open(DATA,$ARGV[0]) or die Couldn t open file: $! ; my $csv = Text::CSV_XS->new(); while(<DATA>) { chomp; $csv->parse($_); my ($id,$ref,$fname,$lname,$country) = $csv->fields; Continued

Pick a naming convention that makes sense when sorted alphabetically. Specifically, when you serialize the version number, you may want to consider using two digits rather than one. If you don t, your file directly might appear as:

Modeling Wavelength Selectivity in Reflection Holography zontal focus equation (]/I ) and vertical focus equation (cos2B/R), it follows that these tools in our shop math toolbox also hold for either transmission or reflection holograms. We just need to be careful to keep track of our angles throughout the entire unit circle and keep our wits about us and keep track of where light really can go.

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